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Extract those 7z files, there will be multiple .bin files and one .cue file. Then go into es_system.cfg and change psx extension to just .cue and .CUE. This is how mine is setup and all my psx roms work.

I tried launching cue files, but didn’t have much luck. Could you give me an example of a game that works (name only)? Or even better, a working game list?

Also, how was performance for your games? The Pi seems to be able to run Quake 3 ok, but I’ve read that PSX games don’t run well.